Plasmonic metamaterial makes a photonic time crystal

Researchers in France and Germany have created the first all-optical photonic time crystal. The nanostructure could be used to make ultrafast optical computers and amplifiers, frequency converters and perhaps even new types of lasers that work in the terahertz range.

Photonic crystals are nanostructured materials with a refractive index that varies on a length scale comparable to the wavelength of light, producing a phenomenon known as a photonic bandgap. This gap affects how photons propagate through the material in a way that resembles how a periodic potential in semiconductors affects the flow of electrons by defining allowed and forbidden energy bands. In the case of photonic crystals, light in certain wavelength ranges can pass through the material, but other wavelengths cannot.

Photonic time crystals (PhTCs) are similar to this, except their properties vary periodically in time, not space. Among other adjustments, this means that instead of photonic bandgaps, they host momentum bandgaps. These gaps are special in that light waves whose momenta fall within them grow exponentially in time.

Optical modulation at THz frequencies

PhTCs show much promise for applications like new types of tuneable lasers and ultrafast frequency converters, but controlling their photonic properties has proven very difficult. This is because these properties need to be modulated very strongly and on ultrashort timescales – on the order of the temporal period of the light itself.

Producing such extremely fast modulations is a key goal for scientists working in a branch of highly nonlinear optics known as time-domain photonics. Previously, their efforts have paid off in the microwave frequency range using PhTCs containing electrical circuits, but all-optical systems have proven elusive.

A team of physicists led by Yannis Laplace of the Ecole Polytechnique in France has now made a PhTC with properties that can be optically modulated at terahertz (THz, 1012 Hz) frequencies. The new PhTC is made from a type of photonic crystal known as a plasmonic metamaterial: an artificially engineered nanostructure consisting of micron-sized cavities made of gold atop an insulating layer and a semiconductor material based on indium and antimony. The cavities trap photons between the gold and semiconductor layers, and surface plasmons – collective, coherent oscillations of conduction electrons that interact very strongly with light – then keep them on the surface of the semiconductor.

Working with scientists from the Collège de France and the Helmholtz-Zentrum Dresden-Rossendorf (HZDR) in Germany, the researchers applied pulses of THz light from the TELBE light source at the HZDR’s ELBE accelerator to their structure. They found that they could use this intense multi-cycle THz light field to modulate the material’s optical properties over timescales of just picoseconds.

Towards new types of lasers in the THz range

“This study builds on previous work in my group related to the development and study of tuneable plasmonic metamaterials in the THz range as a means to create functional devices to control light-matter interactions in this range,” Laplace says. “One of the central questions in our work was to determine if the temporal modulation of the metamaterial would be strong and fast enough.

“By developing a theoretical model in collaboration with our colleague Marco Schiró and his team at the Collège de France that reproduced the experimental observations remarkably well, we showed that the system presented the characteristic spectroscopic signatures expected for a PhTC and provided an explanation for the behaviour of the photons therein.”

The researchers, who detail their work in Nature, also found that the ultrafast temporal modulation reduced the dissipation of photons within the metamaterial by half and they are now looking to reduce these optical losses even further.

“The THz frequency range lies at the junction between electronic and photonic technologies and is historically less developed than these two,” Laplace explains. “With the THz PhTCs that are now achievable, we hope we can soon develop devices like THz amplifiers, frequency converters and maybe new types of THz lasers in this range, hence contributing to the closing of the so-called ‘THz gap,’” he tells Physics World.

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